Bubble geometry

Droge schuim in rust evolueert naar een toestand waar de totale oppervlakte van de schuimbellen is geminimaliseerd. Dit proces veroorzaakt groei bij enkele luchtbellen en inkrimping bij andere. Vijftig jaar geleden toonde John von Neumann aan dat in tweedimensionaal schuim de groeiratio enkel afhangt van het aantal zijden van de polygonale schuimbel. Sascha Hilgenfeldt laat zien dat een goede indicator van de groeiratio in drie dimensies het aantal zijvlakken van de polyhedrale schuimbel is. De analytische theorie en de numerieke simulaties komen bovendien goed overeen

Cracks and fingers: dynamics of ductile fracture in an aqueous foam

Fracture of a quasi-two-dimensional aqueous foam by injection of air can occur via two distinct mechanisms, termed brittle and ductile, which are analogous to crack modes observed for crystalline atomic solids such as metals. In the present work we focus on the dynamics and morphology of the ductile process, in which no films between bubbles are broken. A network modeling approach allows detailed analysis of the foam morphology from individual bubbles to the shape of the propagating crack. This crack develops similarly to fingering instabilities in Hele–Shaw cells filled with homogeneous fluids. We show that the observed width and shape of the crack are compatible this interpretation, and that the discreteness of the bubble structure provides symmetry perturbations and limiting scales characteristic of anomalous fingering. The model thus bridges the gap between fracture of the solid foam lattice and instability growth of interfaces in a fluid system

Sound radiation of 3 MHz driven gas bubbles

The sound radiation of 3 MHz acoustically driven air bubbles in liquid is analysed with respect to possible applications in second harmonic ultrasound diagnostics devices, which have recently come into clinical use. In the forcing pressure amplitude P_a = 1-10 atm and ambient radius R_0 = 0.5-5 \mu m parameter domain a narrow regime around the resonance radius R_0 \sim 1-1.5 \mu m and relatively modest P_a \sim 2-2.5 atm is identified in which optimal sound yield in the second harmonic is achieved while maintaining spherical stability of the bubble. For smaller P_a and larger R_0 hardly any sound is radiated; for larger P_a bubbles become unstable towards non-spherical shape oscillations of their surface. The computation of these instabilities is essential for the evaluation of the optimal parameter regime. A region of slightly smaller R_0 and P_a \sim 1-3 atm is best suited to achieve large ratios of the second harmonic to the fundamental intensity. Spherical stability is guaranteed in the suggested regimes for liquids with an enhanced viscosity compared to water, such as blood.Comment: 19 pages, 10 low resolution ps-figures; higher resolution figures can be retrieved from http://staff-www.uni-marburg.de/~hilgenfe/hires.htm

Analysis of Rayleigh-Plesset dynamics for sonoluminescing bubbles

Recent work on single bubble sonoluminescence (SBSL) has shown that many features of this phenomenon, especially the dependence of SBSL intensity and stability on experimental parameters, can be explained within a hydrodynamic approach. More specifically, many important properties can already be derived from an analysis of bubble wall dynamics. This dynamics is conveniently described by the Rayleigh-Plesset (RP) equation. In this work we derive analytical approximations for RP dynamics and subsequent analytical laws for parameter dependences. These results include (i) an expression for the onset threshold of SL, (ii) an analytical explanation of the transition from diffusively unstable to stable equilibria for the bubble ambient radius (unstable and stable sonoluminescence), and (iii) a detailed understanding of the resonance structure of the RP equation. It is found that the threshold for SL emission is shifted to larger bubble radii and larger driving pressures if surface tension is enlarged, whereas even a considerable change in liquid viscosity leaves this threshold virtually unaltered. As an enhanced viscosity stabilizes the bubbles against surface oscillations, we conclude that the ideal liquid for violently collapsing, surface stable SL bubbles should have small surface tension and large viscosity, although too large viscosity (>40 times the viscosity of water) will again preclude collapses.Comment: 41 pages, 21 eps and ps figures; LaTeX stylefiles replaced because the PostScript file produced at the archive had misplaced and misscaled figure

Predicting the Characteristics of Defect Transitions on Curved Surfaces

The energetically optimal position of lattice defects on intrinsically curved surfaces is a complex function of shape parameters. For open surfaces, a simple condition predicts the critical size for which a central disclination yields lower energy than a boundary disclination. In practice, this transition is modified by activation energies or more favorable intermediate defect positions. Here it is shown that these transition characteristics (continuous or discontinuous, first or second order) can also be inferred from analytical, general criteria evaluated from the surface shape. A universal scale of activation energy is found, and the criterion is generalized to predict transition order as symmetries such as that of the shape are broken. The results give practical insight into structural transitions to disorder in many cellular materials of technological and biological importance

Inert gas accumulation in sonoluminescing bubbles

In this paper we elaborate on the idea [Lohse et al., Phys. Rev. Lett. 78, 1359-1362 (1997)] that (single) sonoluminescing air bubbles rectify argon. The reason for the rectification is that nitrogen and oxygen dissociate and their reaction products dissolve in water. We give further experimental and theoretical evidence and extend the theory to other gas mixtures. We show that in the absence of chemical reactions (e.g., for inert gas mixtures) gas accumulation in strongly acoustically driven bubbles can also occur.Comment: J. Chem. Phys., in press (to appear in November 1997), 30 pages, 15 eps-figure